简介:
邓鹤翔,1985年出生,2007年本科毕业于复旦大学化学系;2011年博士毕业于加州大学洛杉矶分校;2012到2013年先后在加州大学洛杉矶分校和劳伦斯伯克利美国国家实验室开展博士后研究;2013年入选国家级人才计划,加入武汉大学化学与分子科学学院,任教授、博士生导师,现担任学院副院长。2020年获得国家杰出青年科学基金资助。
方向:
研究聚焦CO2吸附、分离与转化中的基础科学问题,设计合成由分子基元构筑的新型晶态孔材料,通过孔径和孔环境的精确定制,在原子及分子尺度上探究CO2与孔材料的相互作用机制,开发原位吸附-小角X射线散射表征新方法,揭示了CO2的吸附、分离行为,并利用光能、电能等可持续性能源实现了CO2的高效转化。在Nature、Nat. Chem.、J. Am. Chem. Soc.等期刊发表论文60余篇。因介孔晶体的研究特色,获得中国分子筛学会于2017年颁发的首届“中国分子筛新秀奖”,2022年霍英东教育基金会高等院校青年科学二等奖。
代表性成果:
1.Molecular Compartments Created in Metal−Organic Frameworks for Efficient Visible-Light-Driven CO2 Overall Conversion. Chengbin Zhao, Zhuo Jiang*, Yin Liu, Yi Zhou, Panchao Yin, Yubin Ke, and Hexiang Deng*, J. Am. Chem. Soc., 2022, doi.org/10.1021/jacs.2c10687
2.Determining Factors in the Growth of MOF Single Crystals Unveiled by in situ Interface Imaging. Jinli Han, Xudong He, Jin Liu, Ruijian Ming, Mohan Lin, Hui Li, Xiaochun Zhou*, Hexiang Deng*, Chem, 2022, 8, 1637-1657.
3.Covalent Organic Frameworks for Optical Applications. Liang Zhang, Lezhi Yi, Zhijun Sun, and Hexiang Deng*, Aggregate, 2021, 2, e24.
4.25 years of Reticular Chemistry. Ralph Freund, Stefano Canossa, Seth M. Cohen, Wei Yan, Hexiang Deng, Vincent Guillerm, Mohamed Eddaoudi, David G. Madden, David Fairen Jimenez, Hao Lyu, Lauren K. Macreadie, Zhe Ji, Yuanyuan Zhang, Bo Wang, Frederik Haase, Christof Wöll, Orysia Zaremba, Jacopo Andreo, Stefan Wuttke* and Christian S. Diercks*, Angew. Chem. Int. Ed., 2021, 60, 23946-23974.
5.Filling Metal-Organic Framework Mesopores with TiO2 for CO2 Photoreduction. Zhuo Jiang†, Xiaohui Xu†, Yanhang Ma, Hae Sung Cho, Deng Ding, Chao Wang, Jie Wu, Peter Oleynikov, Mei Jia, Jun Cheng, Yi Zhou, Osamu Terasaki*, Tianyou Peng, Ling Zan*, and Hexiang Deng*, Nature, 2020, 586, 549-554.
6.Anisotropic Reticular Chemistry. Wentao Xu, Binbin Tu, Qi Liu, Yufei Shu, Cong-Cong Liang, Christian S. Diercks, Omar M. Yaghi*, Yue-Biao Zhang*, Hexiang Deng*, and Qiaowei Li*, Nat. Rev. Mater., 2020, 5, 764-779.
7.Molecular Vises for Precisely Positioning Ligands near Catalytic Metal Centers in Metal-Organic Frameworks. Wei Yan, Shenhui Li*, Tao Yang, Yucong Xia, Xinrui Zhang, Chao Wang, Zier Yan, Feng Deng*, Qianghui Zhou, and Hexiang Deng*, J. Am. Chem. Soc., 2020, 142, 16182-16187.
8.Covalent Organic Framework for Efficient Two-Photon Absorption. Liang Zhang†, Yi Zhou†, Mei Jia†, Yiwen He, Wei Hu, Qi Liu, Jing Li, Xiaohui Xu, Chao Wang, Anna Carlsson, Sorin Lazar, Arno Meingast, Yanhang Ma, Jun Xu, Wen Wen, Zhihong Liu, Jun Cheng, Hexiang Deng*, Matter, 2020, 2, 1049-1063.
9.Efficient Separation of Nucleic Acids with Different Secondary Structures by Metal-Organic Frameworks. Shuang Peng†, Binglin Bie†, Hongnan Jia, Heng Tang, Xiong Zhang, Yuqing Sun, Qi Wei, Fan Wu, Yushu Yuan, Hexiang Deng*, Xiang Zhou*, J. Am. Chem. Soc., 2020, 142, 5049-5059.
10.Metal-Organic Frameworks for the Exploitation of Distance between Active Sites in Efficient Photocatalysis. Xuan Gong†, Yufei Shu†, Zhuo Jiang, Lingxiang Lu, Xiaohui Xu, Chao Wang, Hexiang Deng*, Angew. Chem. Int. Ed., 2020, 59, 5326-5331.
11.Covalent Organic Frameworks as Favorable Constructs for Photodynamic Therapy. Liang Zhang†, Shibo Wang†, Yi Zhou, Chao Wang, Xianzheng Zhang, Hexiang Deng*, Angew. Chem. Int. Ed., 2019, 58, 14213-14218.
12.Isotherms of Individual Pores by Gas Adsorption Crystallography. Hae Sung Cho†, Jingjing Yang†, Xuan Gong†, Yuebiao Zhang, Koichi Momma, Bert M. Weckhuysen, Hexiang Deng*, Jeung Ku Kang, Omar M. Yaghi*, Osamu Terasaki*, Nat. Chem., 2019, 11, 562-570.
13.Nanoscale Laser Metallurgy and Patterning in Air Using MOFs. Haoqing Jiang, Shengyu Jin, Chao Wang, Ruiqian Ma, Yinyin Song, Mengyue Gao, Xingtao Liu, Aiguo Shen, Gary J. Cheng*, Hexiang Deng*, J. Am. Chem. Soc., 2019, 141, 5481-5489.
14.Mesoporous Cages in Chemically Robust MOFs Created by a Large Number of Vertices with Reduced Connectivity. Qi Liu, Yinyin Song, Yanhang Ma, Yi Zhou, Hengjiang Cong, Chao Wang, Jorryn Wu, Gaoli Hu, Michael O’Keeffe, Hexiang Deng*, J. Am. Chem. Soc., 2019, 141, 488-496.
15.Covalent Organic Frameworks Linked by Amine Bonding for Concerted Electrochemical Reduction of CO2. Haoyu Liu, Jun Chu, Zhenglei Yin, Xin Cai, Lin Zhuang, Hexiang Deng*, Chem, 2018, 4, 1696-1709.
16.Molecular Vise Approach to Create Metal‐Binding Sites in MOFs and Detection of Biomarker. Yang Wang†, Qi Liu†, Qin Zhang, Bosi Peng, Hexiang Deng*, Angew. Chem. Int. Ed., 2018, 130, 7238-7243.
17.Metal-organic Frameworks for Precise Inclusion of Single-Stranded DNA and Transfection in Immune Cells. Shuang Peng†, Binglin Bie†, Yangzesheng Sun, Min Liu, Hengjiang Cong, Wentao Zhou, Yucong Xia, Heng Tang, Hexiang Deng*, Xiang Zhou*, Nat. Commun., 2018, 9, 1293.
18.Metal-Organic Frameworks for High Charge-Discharge Rates in Lithium-Sulfur Batteries. Haoqing Jiang†, Xiaochen Liu†, Yushan Wu, Yufei Shu, Xuan Gong, Fusheng Ke*, Hexiang Deng*, Angew. Chem. Int. Ed., 2018, 57, 3916-3921.
19.Multivariate Metal-Organic Frameworks for Dialing-in the Binding and Programming the Release of Drug Molecules. Zhiyue Dong, Yangzesheng Sun, Jun Chu, Xianzheng Zhang, Hexiang Deng*, J. Am. Chem. Soc., 2017, 139, 14209-14216.
20.Principles of Designing Extra-Large Pore Openings and Cages in Zeolitic Imidazolate Frameworks. Jingjing Yang†, Yuebiao Zhang†, Qi Liu, Christopher A. Trickett, Enrique Gutiérrez-Puebla, M. Ángeles Monge, Hengjiang Cong, Abdulrahman Aldossary, Hexiang Deng*, Omar M. Yaghi*, J. Am. Chem. Soc., 2017, 139, 6448-6455.
21.Deciphering the Spatial Arrangement of Metals and Correlation to Reactivity in Multivariate Metal-Organic Frameworks. Qi Liu, Hengjiang Cong, Hexiang Deng*, J. Am. Chem. Soc., 2016, 138, 13822-13825.
22.Extra Adsorption and Adsorbate Superlattice Formation in Metal-Organic Frameworks. Hae Sung Cho†, Hexiang Deng†, Keiichi Miyasaka†, Zhiyue Dong, Minhyung Cho, Alexander V. Neimark, Jeung Ku Kang, Omar M. Yaghi*, Osamu Terasaki*, Nature, 2015, 527, 503-507.
23.Introduction of Functionality, Selection of Topology, and Enhancement of Gas Adsorption in Multivariate Metal-Organic Framework-177. Yue-Biao Zhang, Hiroyasu Furukawa, Nakeun Ko, Weixuan Nie, Hye Jeong Park, Satoshi Okajima, Kyle E. Cordova, Hexiang Deng*, Jaheon Kim*, Omar M. Yaghi*, J. Am. Chem. Soc., 2015, 137, 2641-2650.
24.Large-Pore Apertures in a Series of Metal-Organic Frameworks. Hexiang Deng†, Sergio Grunder†, Kyle E. Cordova, Cory Valente, Hiroyasu Furukawa, Mohamad Hmadeh, Felipe Gándara, Adam C. Whalley, Zheng Liu, Shunsuke Asahina, Hiroyoshi Kazumori, Michael O’Keeffe, Osamu Terasaki, J. Fraser Stoddart, Omar M. Yaghi*, Science, 2012, 336, 1018-1023.
25.Robust Dynamics. Hexiang Deng, Mark A. Olson, J. Fraser Stoddart*, Omar M. Yaghi*, Nature Chem., 2010, 2, 439-443.
26.Multiple Functional Groups of Varying Ratios in Metal-Organic Frameworks. Hexiang Deng, Christian J. Doonan, Hiroyasu Furukawa, Ricardo B. Ferreira, John Towne, Carolyn B. Knobler, Bo Wang, Omar M. Yaghi*, Science, 2010, 327, 846-850.